Direct injection method for determination of 16 kinds of wear elements in lubricating oil - Master's thesis - Dissertation

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WIFI test head can be customized for other specifications


1

Instruments and methods

1.1

Instruments and reagents

Tianrui Instrument

ICP2060T

(Petrochemical-specific) Inductively Coupled Plasma Emission Spectrometer

1.

The semiconductor refrigeration sample introduction device improves the stability and sensitivity of the injection, and the test is more accurate and reliable.

2.

The special torch for gasoline ensures long-term stability of the plasma and reduces the background of the substrate.

3.

Increase oxygen assisted injection to maintain plasma stability and prevent carbon deposits.

1.2

Instrument working conditions

High frequency generator:

27.12MHz

, the center channel is

0.6mm

Quartz torch, high frequency power

1100W

, the reflection power is about

50W

Plasma gas flow

15L/min

Auxiliary gas flow

1.0L/min

Carrier gas flow

0.4L/min

Oxygen flow rate

30ml/min

, spray chamber temperature

-10

°C, peristaltic pump speed

3ml/min

.

1.3

experiment method

After the instrument is automatically ignited and the parameters are set according to the working conditions of the instrument, the diluent directly enters the mist chamber through the atomizer and enters the plasma. After the instrument is stabilized, the blank solution, the standard solution and the diluted sample solution are sequentially measured, and the instrument is operated according to the work. The curve gives the amount of each element in the final sample directly.

1.4

Repeatability test

Continuous test

6

Parallel sample, calculation

6

The relative standard deviation of the test data is the repeatability data. The results are shown in the table below.

element

Repeatability

/RSD

element

Repeatability

/RSD

vanadium(

V

)

1.45%

cadmium(

Cd

)

2.58%

copper(

Cu

)

0.76%

nickel(

Ni

)

2.78%

silver(

Ag

)

0.91%

iron(

Fe

)

1.46%

titanium(

Ti

)

1.35%

silicon(

Si

)

1.70%

barium(

Ba

)

1.48%

manganese(

Mn

)

1.22%

calcium(

Ca

)

1.31%

chromium(

Cr

)

1.10%

Zinc (

Zn

)

1.65%

magnesium(

Mg

)

1.93%

lead(

Pb

)

2.46%

phosphorus(

P

)

2.36%

1.5

Accuracy test

Using this method to test the standard content of the metal content spectrum of lubricating oil

GBW(E)130129

,

GBW(E)130132

Compare the actual measured value with the standard value to obtain the recovery rate of the actual test, and obtain the accuracy data. The results are shown in the table below.

Determination

GBW(E)130129-

Lubricating oil metal content spectral analysis of the results of the reference material (

Mg/kg

)

element

standard value

measured value

Recovery rate

element

standard value

measured value

Recovery rate

vanadium(

V

)

10

9.58

95.8%

cadmium(

Cd

)

10

8.82

88.2%

copper(

Cu

)

10

10.16

101.6%

nickel(

Ni

)

10

9.70

97.0%

silver(

Ag

)

10

9.50

95.0%

iron(

Fe

)

10

9.97

99.7%

titanium(

Ti

)

10

9.97

99.7%

silicon(

Si

)

10

8.25

82.5%

barium(

Ba

)

10

10.73

107.3%

manganese(

Mn

)

10

9.61

96.1%

calcium(

Ca

)

10

10.05

100.5%

chromium(

Cr

)

10

9.41

94.1%

Zinc (

Zn

)

10

10.20

102.0%

magnesium(

Mg

)

10

8.33

83.3%

lead(

Pb

)

10

10.35

103.5%

phosphorus(

P

)

10

10.99

109.9%

Determination

GBW(E)130132-

Lubricating oil metal content spectral analysis of the results of the reference material (

Mg/kg

)

element

standard value

measured value

Recovery rate

element

standard value

measured value

Recovery rate

vanadium(

V

)

100

98.04

98.00%

cadmium(

Cd

)

100

104.91

104.90%

copper(

Cu

)

100

112.57

112.60%

nickel(

Ni

)

100

106.5

106.50%

silver(

Ag

)

100

102.21

102.20%

iron(

Fe

)

100

104.84

104.80%

titanium(

Ti

)

100

102.11

102.10%

silicon(

Si

)

100

91.78

91.80%

barium(

Ba

)

100

118.62

118.60%

manganese(

Mn

)

100

106.09

106.10%

calcium(

Ca

)

100

88.54

88.50%

chromium(

Cr

)

100

99.31

99.30%

Zinc (

Zn

)

100

110.57

110.60%

magnesium(

Mg

)

100

112.43

112.40%

lead(

Pb

)

100

108.39

108.40%

phosphorus(

P

)

100

97.81

97.80%



2 .

in conclusion

Injection with inorganic digestion solution

ICP

Compared with the law,

ICP

The organic injection method has an absolute advantage in analysis speed. The optimization of the working conditions of the instrument is guaranteed

ICP

The key to accurate analysis of organic injection methods. Organic injection method with good accuracy and repeatability

,

Can meet the analysis requirements. It is suitable for accurate testing of batch samples. The detection results have good detection limits, accuracy and repeatability, and are suitable for popularization in the petrochemical industry.

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